| 上海市大气气溶胶散射系数的季节变化特征 |
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| 作者姓名： | 徐薇 修光利 陶俊 朱梦雅 蔡婧 王丽娜 张仁健 |
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| 作者单位： | 1. 华东理工大学国家环境保护化工过程环境风险评价与控制重点实验室, 上海 200237;
2. 环保部华南环境科学研究所, 广州 510653;
3. 中国科学院大气物理研究所大气边界层物理和大气化学国家重点实验室, 北京 100029 |
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| 基金项目： | 国家自然科学基金（21277044）、国家环境保护公益性科研专项（200809143）、中央高校基本科研专项（WB1113005）、上海市教委科研创新基金（12ZZ054）和博士点基金（20120074140001）等资助 |
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| 摘 要： | 2009年4—12月于华东理工大学某实验楼楼顶利用浊度仪对大气散射系数进行监测，同时采集获得PM2.5质量浓度，分析其成分组成和不同季节散射系数日变化特征、散射系数与PM2.5的相关性，以及大气能见度与PM2.5成分的幂函数关系.结果表明，散射系数秋、冬季较高，夏季最小.日变化特征在6：00和18：00各出现1个峰值，秋、冬季晚高峰较显著，夏季日变化较平缓；4个季节比较，PM2.5质量浓度与散射系数均呈现良好线性关系；春季大气能见度与PM2.5中二次离子呈显著幂函数相关性，夏季能见度与EC相关性显著，秋季能见度与有机物和二次离子均呈显著性幂相关，冬季能见度与各组分关系不显著.
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| 关 键 词： | 散射系数 能见度 PM2.5" target="_blank">2.5')">PM2.5 |
| 收稿时间： | 2013-05-31 |
| 修稿时间： | 2013-11-06 |
Seasonal variation characteristics of atmospheric aerosol scattering coefficients in Shanghai |
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| Authors: | XU Wei XIU Guangli TAO Jun ZHU Mengya CAI Jing WANG Lina ZHANG Renjian |
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| Institution: | 1. State Environmental Protection Key Laboratory of Risk Assessment and Control on Chemical Processes, East China University of Science and Technology, Shanghai 200237, China;
2. Ministry of South China Environmental Science Research Institute, Guangzhou 510653, China;
3. Key Laboratory of Regional Climate-Environment for Temperate East Asia(RCE-TEA), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China |
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| Abstract: | We used a nephelometer to monitor scattering coefficients on the top of a laboratory building in East China University of Science and Engineering from April to December in 2009. PM2.5 was simultaneously sampled every day to obtain its mass concentrations and its chemical components. We studied characteristics of diurnal variation in scattering coefficients in different seasons, correlations between scattering coefficient and PM2.5, and power correlation between visibility and chemical components of PM2.5. Results indicated that scattering coefficients were higher in autumn and winter and lower in summer. The diurnal variation of scattering coefficient indicated two peaks observed at 6:00 and 18:00,respectively. The peak value was higher in autumn and winter but the diurnal variation changed little in summer. The seasonal comparison indicated that scattering coefficients had strong linear correlations with PM2.5 in all the seasons. It was found that visibility had power function correlations with secondary ions in spring, with EC in summer, and with both organic components and secondary ions in fall. Due to the complexity of components, sources, and formation mechanisms, no obvious correlations between visibility and components were found for winter. |
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| Keywords: | scattering coefficients visibility 2 PM2" target="_blank">5')">PM2 5 |
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