Surface modification of ZnIn2S4 layers to realize energy-transfer-mediated photocatalysisOA |
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作者姓名: | Xianshun Sun Xiao Luo Sen Jin Xiaodong Zhang Hui Wang Wei Shao Xiaojun Wu Yi Xie |
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作者单位: | 1. Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China;2. Institute of Energy, Hefei Comprehensive National Science Center |
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基金项目: | supported by the National Key R&D Program of China (2019YFA0210004);;the National Natural Science Foundation of China (21922509,92163105, T2122004, 21905262, 21890754, U2032212 and U2032160);;the fellowship of China Postdoctoral Science Foundation (2020M682011);;the Fundamental Research Funds for the Central Universities(WK2060000035); |
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摘 要: | Photocatalytic selective aerobic oxidation reactions are crucial in designing advanced organic intermediates,but suffer from low conversion efficiency.Hence,activating 1O2 to create suitable reactive oxygen species,such as singlet oxygen(1O2),can significantly increase the yield of desired products.Herein,using ZnIn2S4 nanosheets as a model system,we build a surface-modified theoretical structure,where a surface-covered non-conduc...
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