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Surface modification of ZnIn2S4 layers to realize energy-transfer-mediated photocatalysisOA
作者姓名:Xianshun Sun  Xiao Luo  Sen Jin  Xiaodong Zhang  Hui Wang  Wei Shao  Xiaojun Wu  Yi Xie
作者单位:1. Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China;2. Institute of Energy, Hefei Comprehensive National Science Center
基金项目:supported by the National Key R&D Program of China (2019YFA0210004);;the National Natural Science Foundation of China (21922509,92163105, T2122004, 21905262, 21890754, U2032212 and U2032160);;the fellowship of China Postdoctoral Science Foundation (2020M682011);;the Fundamental Research Funds for the Central Universities(WK2060000035);
摘    要:Photocatalytic selective aerobic oxidation reactions are crucial in designing advanced organic intermediates,but suffer from low conversion efficiency.Hence,activating 1O2 to create suitable reactive oxygen species,such as singlet oxygen(1O2),can significantly increase the yield of desired products.Herein,using ZnIn2S4 nanosheets as a model system,we build a surface-modified theoretical structure,where a surface-covered non-conduc...

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